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One Piece: Grand Adventure

Unlock Eneru (Crocodile's adventure mode)
Get Eneru as your ally in the Jaya area and win a battle using him.

Unlock Mihawk (Chaser's adventure mode)
After recruiting Mihawk win a battle using him.

Unlock Mr. 2 Bon Clay (Crocodile's adventure mode)
Get Mr. 2 as your ally and win a battle using him.

Unlock Nico Robin (Luffy's adventure mode)
Get her as your ally at the end and win a battle using her.

Unlock Ohm (Crocodile's adventure mode)
Get Ohm as your ally in the Jaya area and win a battle using him.

Unlock Shanks (Buggy's adventure mode)
Recruit Shanks and then win a battle using him.

Unlock Trace (Buggy's adventure mode)
Recruit him in Drum Island then win a battle using him

Buggy:
Reach the "Top Pirate of the Island" rank to unlock Buggy as a captain in Grand Adventure mode.

Chaser:
Reach level 15 with him in Chaser's adventure, then win a battle using him.

Chaser (Smoker):
Get the "Top Pirate of the Grand Line" rank to unlock Chaser (Smoker) as a captain in Grand Adventure mode.

Crocodile:
Get the "Top Pirate of the Continent" rank to unlock Crocodile as a captain in Grand Adventure mode. 

Kuina:
In Adventure mode as Chaser, recruit Kuina in the ship graveyard. Then, defeat Zolo using her in Alabasta. .

Ussop:
Defeat the final boss in Adventure mode as Luffy, Buggy, Crocodile, and Chaser in any order.

Zeff:
In Adventure mode as Chaser, get Zeff to level 15 and use him once in battle.

Support characters in Grand Battle mode:
Use a support character for three battles in Adventure mode, and they can be used by any character in Grand Battle mode.

Versus mode passwords:
Enter the following case-sensitive passwords to unlock the corresponding level 100 character in Versus mode.